Look through your healthiest nasturtium plants with your hands to find green seed pods, which grow to about 1/3 inch in diameter. Nasturtium seed pods often grow in groups of three or four. Pull or snip off the plumpest pods with hand clippers.
Spread the seed pods on newspaper or a cookie tray. Set them in a dry, well-ventilated area of your home for one or two weeks until they dry completely and turn brown.
Separate the seeds from the pods. The pods should open up during the drying process. Take the seeds out with your fingers.
Throw out other debris and the pods and store the seeds in a paper bag or airtight containers like old jelly or olive jars. Place them in a cool and dark location like your garage or in the bottom drawer of your refrigerator.