Paint or stain the molding pieces. Use a high-quality latex or oil-based paint or a thick gel stain. Do not use a semitransparent stain; it is too thin and will not cover the urethane molding. Apply the paint or stain to match existing trim with a 1-inch-wide paintbrush, carefully covering all the molding detail. Allow the molding to dry thoroughly.
Nail all the inside corner pieces in place. Use shims, if necessary, to fill in gaps where corners are not square.
Nail in all the outside corner pieces, using the same procedure as in Step 2.
Measure the distance between one pair of corner blocks. Add 1/8 inch to this measurement and cut the crown molding with a handsaw to match.
Push one end of the molding against a corner piece. Flex the molding a bit to make it to fit against the other corner piece. Press the molding gently until it snaps into place.
Find the wall studs using a stud finder. Hammer the molding to the wall using a 2-inch finishing nail on every other stud.
Insert a nail into the ceiling joist every 3 feet. If your ceiling joists run parallel to the molding, hammer a nail on an angle into the drywall or plaster every 3 feet.
Install the remaining molding to fit between corner pieces or divider blocks following Steps 4 through 7.
Fill any gaps along the wall and the ceiling using colored caulk.
Fill all nail holes with a crayon-style putty stick. Wipe away any excess putty with a damp cloth.